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• W4309810318 startingPage "22295" @default.
• W4309810318 abstract "Hydrochromic materials characterized by noticeable color change upon water exposure have attracted pervasive attention for their frontier applications in sensing and information technologies. However, existing hydrochromic materials typically suffer from a slow hydrochromic response as well as limited stability and color tunability. This work describes a novel hydrochromic perovskite crystal composed of zero-dimensional Cs3TbF6:Eu3+, which displays switchable luminescence due to the constituent Tb3+ and Eu3+ ions. Mechanistic investigation reveals that the hydrochromic property stems from a water-induced phase transformation into a one-dimensional structure through a CsF-stripping process. The phase transformation triggers energy coupling between Tb3+ and Eu3+ ions in adjacent lanthanide halide polyhedra, resulting in an emission color change from green to orange. Notably, the phase transformation is ultrafast (20 ms) and reversible, and the emission color in each phase can be fine-tuned by controlling the Eu3+ doping concentration along with Y3+ co-doping. The advances in these hydrochromic luminescent materials offer exciting opportunities for information security and data storage." @default.
• W4309810318 created "2022-11-29" @default.
• W4309810318 creator A5026518307 @default.
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• W4309810318 date "2022-11-23" @default.
• W4309810318 modified "2023-10-16" @default.
• W4309810318 title "Ultrafast and Multicolor Luminescence Switching in a Lanthanide-Based Hydrochromic Perovskite" @default.
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• W4309810318 doi "https://doi.org/10.1021/jacs.2c10809" @default.
• W4309810318 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36417793" @default.
• W4309810318 hasPublicationYear "2022" @default.
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