Matches in SemOpenAlex for { <https://semopenalex.org/work/W4310010102> ?p ?o ?g. }
- W4310010102 abstract "Abstract The combined catalytic systems derived from organocatalysts and transition metals exhibit powerful activation and stereoselective-control abilities in asymmetric catalysis. This work describes a highly efficient chiral aldehyde-nickel dual catalytic system and its application for the direct asymmetric α−propargylation reaction of amino acid esters with propargylic alcohol derivatives. Various structural diversity α,α−disubstituted non-proteinogenic α−amino acid esters are produced in good-to-excellent yields and enantioselectivities. Furthermore, a stereodivergent synthesis of natural product NP25302 is achieved, and a reasonable reaction mechanism is proposed to illustrate the observed stereoselectivity based on the results of control experiments, nonlinear effect investigation, and HRMS detection." @default.
- W4310010102 created "2022-11-30" @default.
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- W4310010102 date "2022-11-26" @default.
- W4310010102 modified "2023-10-14" @default.
- W4310010102 title "Chiral aldehyde-nickel dual catalysis enables asymmetric α−propargylation of amino acids and stereodivergent synthesis of NP25302" @default.
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- W4310010102 doi "https://doi.org/10.1038/s41467-022-35062-2" @default.
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