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- W4310082982 abstract "The McMurry coupling is a facile, gentle and low-cost chemical reaction for synthesizing. Here, for the first time, we employed the McMurry coupling reaction to prepare π-conjugated anion exchange membranes (AEMs). The inter-chain π-π stacking between adjacent benzene rings induces directional self-assembly aggregation and enables highly ordered ion-conductive channels. The resulting structure was characterized through UV/VIS spectrum, X-ray diffraction (XRD) pattern, small-angle X-ray scattering (SAXS), transmission electron microscopy (TEM) and density functional theory (DFT) calculations, leading to high OH− conductivity of 135.5 mS cm−1 at 80 °C. Furthermore, the double bonds in the π-conjugated system also trigger in situ self-crosslinking of the AEMs to enhance dimensional and alkaline stability. Benefiting from this advantage, the as-obtained Cr-QPPV-2.51 AEM exhibits superior alkaline stability (95 % conductivity retention after 3000 hrs in 1 M KOH at 80 °C) and high mechanical strength of 34.8 MPa. Moreover, the fuel cell using Cr-QPPV-2.51 shows a maximum peak power density of 1.27 W cm−2 at 80 °C." @default.
- W4310082982 created "2022-11-30" @default.
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- W4310082982 date "2022-12-14" @default.
- W4310082982 modified "2023-10-18" @default.
- W4310082982 title "A π‐Conjugated Anion‐Exchange Membrane with an Ordered Ion‐Conducting Channel via the McMurray Coupling Reaction" @default.
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- W4310082982 doi "https://doi.org/10.1002/anie.202215017" @default.
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