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- W4310263708 abstract "The bismuth oxide (BiOx) derived electrocatalysts hold the promise for effective carbon dioxide (CO2) reduction to formate as liquid fuel. However, the disappearance of the active edge sites during the electroreduction, due to the spontaneous aggregation of nanoclusters into large sheets, lowers the performance at high current densities. Here we develop a ligand-confined strategy to stabilize Bi-BiOx nanodots with a diameter of ca. 5 nm, enabling efficient CO2 reduction to formate with high activity (working current density up to 1 A/cm2) and high selectivity (Faradaic efficiency of >95 %). We find that the poly(methacrylic acid) ligand would in-situ transform into carbon shell as a confinement area that limits the growth of Bi-BiOx nanodots, thus keeping the abundant active edge sites for CO2 reduction at wide working potentials. We also note that the carboxyl group in ligand remained on nanodots may provide oxygen donors for Bi-BiOx to maintain the selective formate generation at high current densities." @default.
- W4310263708 created "2022-11-30" @default.
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- W4310263708 date "2023-03-01" @default.
- W4310263708 modified "2023-10-09" @default.
- W4310263708 title "Ligand-confined bismuth based nanodots for robust carbon dioxide reduction to liquid fuel at 1 A/cm2" @default.
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- W4310263708 doi "https://doi.org/10.1016/j.ces.2022.118354" @default.
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