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• W4310276887 abstract "Abstract The electrocatalytic nitrogen reduction reaction (NRR) provides a promising avenue for sustainable and decentralized green ammonia (NH 3 ) synthesis. To promote the NRR, the design and synthesis of efficient electrocatalysts with an elucidated reaction mechanism is critically important. Here, surface hydrogenation‐facilitated NRR is demonstrated to yield NH 3 at low overpotentials on oxygen‐deficient In 2 O 3 plates decorated with single atom CdO 5 that have a weak N 2 ‐binding capability. Adsorbed * H is calculated to be first produced via the Volmer reaction (H 2 O + e − → * H + OH − ) and then reacts with dissolved N 2 to generate * N 2 H 2 , which is likely the rate determining step (RDS) of the whole process. Cd atoms and oxygen vacancies in In 2 O 3 jointly enhance the activation of N 2 and accelerate the RDS, boosting the NRR. An NH 3 production rate of as high as 57.5 µg h −1 mg cat −1 is attained at a mild potential, which is retained to a large extent even after 44 h of continuous polarization." @default.
• W4310276887 created "2022-11-30" @default.
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• W4310276887 date "2022-11-27" @default.
• W4310276887 modified "2023-10-16" @default.
• W4310276887 title "Pre‐Adsorbed H‐Assisted N ₂ Activation on Single‐Atom Cadmium‐O ₅ Decorated In ₂ O ₃ for Efficient NH ₃ Electrosynthesis" @default.
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• W4310276887 doi "https://doi.org/10.1002/adfm.202209843" @default.
• W4310276887 hasPublicationYear "2022" @default.
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