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- W4310359059 abstract "In this work, monodisperse β-NaLuF4:Yb,Er microcrystals with intense upconversion emission were synthesized via a modified hydrothermal method. With the increase of reactant concentration, their production yield is increased obviously, and the upconversion emission intensity in β-NaLuF4:Yb,Er microcrystals is also enhanced significantly. The luminescence enhancement should be attributed to minimal internal OH− defects, validated by a combination of analytical X-ray diffraction (XRD), energy dispersive spectrum (EDS), and Eu3+ structural probe measurements. We also reveal that high Na+:RE3+ ratio in the β-NaLuF4:Yb,Er microcrystals prepared under Na+-rich reaction will arouse the increased repulsive energy of β-NaLuF4 microcrystals between F− and OH− anions and then facilitate the substitution of large OH− ions by small F− ions under F−-rich reaction conditions. Minimal OH− concentrations can limit nonradiative relaxation and promote excitation energy harvesting for high upconversion efficiency. The presented results not only offer a facile method for the simultaneous production yield and luminescence intensity increase of β-NaREF4 microcrystals, but also uncover a better insight into the upconversion emission alterations, which is favorable to broaden their practical applications." @default.
- W4310359059 created "2022-12-09" @default.
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- W4310359059 date "2023-04-01" @default.
- W4310359059 modified "2023-10-17" @default.
- W4310359059 title "One-pot synthesis of hexagonal NaLuF4:Yb,Er microcrystals with enhanced upconversion emission and high production yield" @default.
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- W4310359059 doi "https://doi.org/10.1016/j.jre.2022.11.014" @default.
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