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- W4310376612 abstract "Can commodity polymers are made to be healable just by blending with self-healable polymers? Here we report the first study on the fundamental aspect of this practically challenging issue. Poly(ether thiourea) (PTUEG3 ; Tg =27 °C) reported in 2018 is extraordinary in that it is mechanically robust but can self-heal even at 12 °C. In contrast, poly(octamethylene thiourea) (PTUC8 ; Tg =50 °C), an analogue of PTUEG3 , cannot heal below 92 °C. We found that their polymer blend self-healed in a temperature range above 32 °C even when its PTUEG3 content was only 20 mol %. Unlike PTUEG3 alone, this polymer blend, upon exposure to high humidity, barely plasticized, keeping its excellent mechanical properties due to the non-hygroscopic nature of the PTUC8 component. CP/MAS 13 C NMR analysis revealed that the polymer blend was nanophase-separated, which possibly accounts for why such a small amount of PTUEG3 provided the polymer blend with humidity-tolerant self-healable properties." @default.
- W4310376612 created "2022-12-10" @default.
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- W4310376612 date "2022-12-20" @default.
- W4310376612 modified "2023-10-16" @default.
- W4310376612 title "Blending to Make Nonhealable Polymers Healable: Nanophase Separation Observed by CP/MAS <sup>13</sup> C NMR Analysis" @default.
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- W4310376612 doi "https://doi.org/10.1002/anie.202214444" @default.
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