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• W4310377008 abstract "As rising star materials, single-atom and dual-atom catalysts have been widely reported in the electro-catalysis area. To answer the key question: single-atom and dual-atom catalysts, which is better for electrocatalytic urea synthesis? we design two types of catalysts via a vacancy-anchorage strategy: single-atom Pd1−TiO2 and dual-atom Pd1Cu1−TiO2 nanosheets. An ultrahigh urea activity of 166.67 molurea molPd−1 h1 with the corresponding 22.54 % Faradaic efficiency at −0.5 V vs. reversible hydrogen electrode (RHE) is achieved over Pd1Cu1−TiO2, which is much higher than that of Pd1−TiO2. Various characterization including an in situ diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS) and theoretical calculations demonstrate that dual-atom Pd1Cu1 site in Pd1Cu1−TiO2 is more favorable for producing urea, which experiences a C−N coupling pathway with a lower energy barrier compared with Pd1 in Pd1−TiO2." @default.
• W4310377008 created "2022-12-10" @default.
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• W4310377008 date "2023-01-13" @default.
• W4310377008 modified "2023-10-11" @default.
• W4310377008 title "Single‐Atom or Dual‐Atom in TiO ₂ Nanosheet: Which is the Better Choice for Electrocatalytic Urea Synthesis?" @default.
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• W4310377008 doi "https://doi.org/10.1002/anie.202216835" @default.
• W4310377008 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36448542" @default.
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