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- W4310490405 abstract "Two π-conjugated trithiocyanurates A(H2C3N3S3) (A = NH4, Cs) were successfully synthesized via a mild aqueous solution method or hydrothermal technique, and the ammonium bicarbonate and cesium hydroxide were used as deprotonation agents. NH4(H2C3N3S3) crystallizes in a symmetric space group P1̅ with flat [H2C3N3S3]∞ chain separated by NH4+, whereas Cs(H2C3N3S3) belongs to an asymmetric space group Cc [Z = 4, a = 5.405(6) Å, b = 21.263(3) Å, c = 14.996(2) Å, β = 92.408(10)°] with wavy [H2C3N3S3]∞ chain separated by Cs+. More importantly, Cs(H2C3N3S3) displays a strong second-harmonic generation effect (4.6 × KH2PO4), a large birefringence (Δn = 0.196@1064 nm), and a thermal stability up to 271.3 °C. In addition, a theoretical study further reveals that the π-conjugated (H2C3N3S3)− group has made a primary contribution toward enhancing the linear and nonlinear optical properties in the above two compounds." @default.
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- W4310490405 date "2022-12-01" @default.
- W4310490405 modified "2023-10-14" @default.
- W4310490405 title "Explorations of Second-Order Nonlinear Optical Materials in the Monovalent Trithiocyanurate System" @default.
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- W4310490405 doi "https://doi.org/10.1021/acs.cgd.2c01050" @default.
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