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- W4310570043 abstract "Organic-inorganic perovskite solar cells (PSCs) have achieved great attention due to their expressive power conversion efficiency (PCE) up to 25.7%. To improve the photovoltaic performance of PSCs, interface engineering between the perovskite and hole transport layer (HTL) is a widely used strategy. Following this concept, benzyl trimethyl ammonium chlorides (BTACls) are used to modify the wet chemical processed perovskite film in this work. The BTACl-induced low dimensional perovskite is found to have a bilayer structure, which efficiently decreases the trap density and improves the energy level alignment at the perovskite/HTL interface. As a result, the BTACl-modified PSCs show an improved PCE compared to the control devices. From device modeling, the reduced charge carrier recombination and promoted charge carrier transfer at the perovskite/HTL interface are the cause of the open-circuit (Voc ) and fill factor (FF) improvement, respectively. This study gives a deep understanding for surface modification of perovskite films from a perspective of the morphology and the function of enhancing photovoltaic performance." @default.
- W4310570043 created "2022-12-12" @default.
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- W4310570043 date "2022-12-01" @default.
- W4310570043 modified "2023-10-14" @default.
- W4310570043 title "Deciphering the Morphology Change and Performance Enhancement for Perovskite Solar Cells Induced by Surface Modification" @default.
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- W4310570043 doi "https://doi.org/10.1002/advs.202205342" @default.
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