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- W4310677447 abstract "Developing bifunctional electrodes for oxidation catalysis is highly desirable for hydrogen and value-added chemicals production. Herein, we directly activate the nickel foam through the incorporation of elemental P (P-NF) using a facile, controllable, and ultrafast in-liquid plasma electrolysis approach. When serving for oxygen evolution reaction (OER) in 1 M KOH at room temperature, the optimized P-NF can afford 500 mA cm−2 at 350 mV, and stabilize this current density for over 120 h. Remarkably, the electrode maintains a stable industrial-grade current density in an assembled electrolyzer under quasi-industrial conditions (60 ℃ and 6 M KOH) for over 107 h. The combination of ex/in-situ characterizations and theoretic calculations unequivocally illustrates that P-incorporation induces an elevated electrode porosity and wettability, increased and immobilized Fe impurity doping, as well as enhanced conductivity, forming active Fe-doped γ-NiIIIOOH during OER. The practical bifunctionality of P-NF is additionally verified with selective oxygenation of organics forming value-added chemicals." @default.
- W4310677447 created "2022-12-15" @default.
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- W4310677447 date "2023-05-01" @default.
- W4310677447 modified "2023-10-14" @default.
- W4310677447 title "Activation of nickel foam through in-liquid plasma-induced phosphorus incorporation for efficient quasi-industrial water oxidation and selective oxygenation of organics" @default.
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- W4310677447 doi "https://doi.org/10.1016/j.apcatb.2022.122249" @default.
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