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- W4310851876 abstract "Dry reforming of methane (DRM) is a prospective technology for efficient utilization of CH4 and CO2, with the essential challenge being the design and synthesis of efficient catalysts. In this research, serial encapsulated Ni-based catalysts ([email protected], x = 5, 7, 10) by silica zeolite (S-1) were prepared successfully. The effects of support structure, preparation method and Ni content upon the catalytic performance for DRM were investigated and diverse characterizations were utilized for revealing structural features of as-prepared catalysts. Encapsulated [email protected] catalyst prepared using the one-pot hydrothermal method could acquire more homogeneously dispersed metallic Ni particles and more Ni species including Ni0, NiO, 1:1/2:1 Ni phyllosilicates that could facilitate forming stable Ni0 sites and Ni2+-O2- ion pairs for adsorption and activation of CH4 and CO2, respectively. Hence, [email protected] still maintained the highest CH4 and CO2 conversions of 57.9% and 88.6% and H2/CO molar ratio of 0.90 after 52 h stability tests." @default.
- W4310851876 created "2022-12-19" @default.
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- W4310851876 date "2023-03-01" @default.
- W4310851876 modified "2023-10-10" @default.
- W4310851876 title "Dry reforming of methane over silica zeolite-encapsulated Ni-based catalysts: Effect of preparation method, support structure and Ni content on catalytic performance" @default.
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- W4310851876 doi "https://doi.org/10.1016/j.ijhydene.2022.11.167" @default.
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