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- W4310961457 abstract "In this report, we present a highly efficient approach for the synthesis of β,γ-disubstituted γ-butyrolactone motifs. This newly developed strategy is based on the combination of a diastereoselective aldol and a nickel carbene-mediated γ-butyrolactonization and uses an effective intramolecular ring closure to rapidly access a range of functionalized chiral γ-butyrolactones. This single-step approach was applied to produce straightforward asymmetric syntheses of (−)-talaumidin methyl ether, (+)-veraguensin, and (+)-dubiusamine A and a formal synthesis of (+)-phaseolinic acid as one of the shortest syntheses disclosed to date." @default.
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- W4310961457 date "2022-12-08" @default.
- W4310961457 modified "2023-10-16" @default.
- W4310961457 title "Nickel Carbene-Mediated One-Carbon Homologative γ-Butyrolactonization" @default.
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- W4310961457 doi "https://doi.org/10.1021/acs.orglett.2c03800" @default.
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