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• W4311236633 abstract "The photocatalytic conversion of soluble U(VI) into insoluble U(IV) is a robust strategy to harvest aqueous uranium, but remains challenging owing to the intermittent availability of solar influx and reoxidation of U(IV) without illumination. Herein, a dual platform based on K+ and cyano group co-decorated poly(heptazine imide) (K-CN-PHI) is reported that can drive persistent U(VI) extraction upon/beyond light. K-CN-PHI achieves the photocatalytic reduction of U(VI) with a reaction rate of 0.89 min-1 , being 47 times greater than that over pristine carbon nitride (PCN). This system can further be triggered by light to form long-living radicals, driving the reduction of U(VI) in the dark for over 3 d. The flexible structural K+ as counterions stabilize the electrons trapped by cyanamide groups, enabling the long lifetime of the generated radicals. The results collectively prove K-CN-PHI to be a novel and efficient photocatalyst enabling persistent U(VI) extraction around the clock, and broadening the practical applications of the photocatalytic extraction of U(VI)." @default.
• W4311236633 created "2022-12-24" @default.
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• W4311236633 date "2022-12-13" @default.
• W4311236633 modified "2023-09-30" @default.
• W4311236633 title "New Strategy for the Persistent Photocatalytic Reduction of U(VI): Utilization and Storage of Solar Energy in K⁺ and Cyano Co‐Decorated Poly(Heptazine Imide)" @default.
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• W4311236633 doi "https://doi.org/10.1002/advs.202205542" @default.
• W4311236633 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36511158" @default.
• W4311236633 hasPublicationYear "2022" @default.
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