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• W4311267980 abstract "Abstract Interface plays an important role in determining the optoelectronic properties of perovskite film to access efficiency photovoltaic device. Herein, a functional molecular with two-terminal donor groups was deposited between the SnO 2 electron transport layer and halide perovskite to manipulate the perovskite crystal growth and passivate defects at the interface. It’s found that isonicotinohydrazide (INHA) can anchor Pb 2+ cluster in precursor against the harsh perovskite ingredient exhaustion, leading to a uniform nuclei distribution for crystal growth in the whole perovskite film. Growth manipulation give rise to confinement induced dynamical crystallization process leading a uniform perovskite film from bottom to top. As well, more analysis shows that interfacial modification can greatly reduce trap defects and therefore facilitate photogenerated carrier-transferring. The efficient electron transfer and reduced interface traps correlate well with the corresponding fill factors and open-circuit voltages (V OC ) of working devices. The resulting perovskite solar cell exhibits striking improvements to reach the champion efficiency of 21.12%. The long-term stability is also significantly enhanced compared to pristine devices. This work highlights the origin of INHA/perovskite interfacial interaction and offer a growth model for further perfecting perovskite films." @default.
• W4311267980 created "2022-12-25" @default.
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• W4311267980 date "2022-12-13" @default.
• W4311267980 modified "2023-10-14" @default.
• W4311267980 title "Buried-in Interface with Two-terminal Functional Groups for Perovskite- based Photovoltaic Solar Cells" @default.
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• W4311267980 doi "https://doi.org/10.21203/rs.3.rs-2318901/v1" @default.
• W4311267980 hasPublicationYear "2022" @default.
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