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- W4311346025 abstract "Abstract Ammonia (NH 3 ) has the characteristics of large hydrogen content and high energy density, which is in line with the concept of green and low-carbon circular economic development. Since nitrogen (N 2 ) sources are abundant on earth, they can be used to synthesize NH 3 . The critical step is breaking the N≡N bond (945 kJ/mol), and then activating N 2 . Today, industry requires the production of NH 3 at the temperature as high as 300-500°C and the pressure as high as 150-300 atm, using metal catalysts such as iron (Fe) or ruthenium (Ru), which consumes plenty of energy. The electrocatalytic nitrogen reduction reaction is considered to be an alternative expected method for NH 3 production under gentle conditions, in which the catalysis of the electrocatalyst plays a crucial role. The results indicate that N 2 can be effectively enabled by B/WS 2 and can accelerate the process which converts nitrogen gas into ammonia through an alternative mechanism of nitrogen reduction reaction (NRR) in a low limiting potential of -0.44 V. Furthermore, the as-designed catalyst performed highly thermodynamic stable, highly active, and highly NRR select. Thus, this work gives researchers a new perspective on N 2 fixation by lower dimensional electrocatalyst materials under gentle conditions." @default.
- W4311346025 created "2022-12-25" @default.
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- W4311346025 date "2022-12-01" @default.
- W4311346025 modified "2023-10-14" @default.
- W4311346025 title "Doped single B atom on WS<sub>2</sub> as a promising electrocatalyst" @default.
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- W4311346025 doi "https://doi.org/10.1088/1742-6596/2390/1/012039" @default.
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