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- W4311360314 endingPage "156050" @default.
- W4311360314 startingPage "156050" @default.
- W4311360314 abstract "For this study, a WO3/Bi5O7I direct Z-scheme heterojunction material was successfully synthesized via a solvothermal-calcination method. The WO3/Bi5O7I heterostructure enhanced the absorption of light and accelerated the separation of charge carriers. Under simulated sunlight irradiation, the removal rate of rhodamine B (RhB) reached 99.6% over the optimal WB14 composite (mass ratio of WO3: Bi5O7I was 14%), which was 2.53 and 30 times that of pristine Bi5O7I and WO3, respectively. Experimental parameters including the WB14 dosage, initial RhB concentration, solution pH, and water sources were explored. Meanwhile, the WB14 exhibited excellent stability and reusability under simulated sunlight. The degradation pathway of RhB was speculated and the toxicity of intermediates was evaluated using the ECOSAR program. Moreover, tetracycline (TC) was employed as a common antibiotic to verify the universality of the catalysts. Capturing experiments and electron paramagnetic resonance (EPR) tests revealed that h+ served as the main active species in the photocatalysis, while OH and O2– played secondary roles. Finally, the formation of Z-scheme heterojunctions between the Bi5O7I and WO3 was inferred based on charge carrier migration and reactive species in the photocatalytic system. This study provides insights into the design of Z-scheme heterojunctions, which is helpful toward the development of Z-scheme heterojunction concepts." @default.
- W4311360314 created "2022-12-25" @default.
- W4311360314 creator A5021678671 @default.
- W4311360314 creator A5023636900 @default.
- W4311360314 creator A5027534949 @default.
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- W4311360314 creator A5045634141 @default.
- W4311360314 creator A5051900876 @default.
- W4311360314 creator A5071880985 @default.
- W4311360314 creator A5079650655 @default.
- W4311360314 creator A5082251778 @default.
- W4311360314 date "2023-03-01" @default.
- W4311360314 modified "2023-10-18" @default.
- W4311360314 title "Synthesis of 2D/2D direct Z-scheme WO3/Bi5O7I heterojunctions for decomposition and detoxification of organic compounds under simulated sunlight" @default.
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