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- W4311361715 abstract "Abstract A series of novel 3‐ N , N ‐dimethylaminofunctionalized phosphinines were synthesized and structurally characterized. DFT calculations showed that these aromatic phosphorus heterocycles possess stronger π‐donor and σ‐donor properties compared to the parent phosphinine C 5 H 5 P. With CuBr ⋅ SMe 2 , the corresponding complexes of the type [(phosphinine) 2 CuBr] 2 are formed, which show the classical terminal σ‐coordination mode of the phosphorus donor towards the Cu(I) center. Upon reaction with AuCl ⋅ SMe 2 , mononuclear phosphinine‐Au(I)Cl complexes could be obtained and crystallographically characterized. Moreover, the presence of a SiMe 3 ‐group and a donor‐functionality provide the possibility for post‐synthetic ligand modifications. With CuCl ⋅ SMe 2 the phosphinine‐based hydrochloride salts forms a rare Cu(I) complex with a Cu 4 Cl 4 ‐core, that contains two pairs of differently coordinating phosphinine ligands." @default.
- W4311361715 created "2022-12-25" @default.
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- W4311361715 date "2022-12-27" @default.
- W4311361715 modified "2023-10-18" @default.
- W4311361715 title "Copper(I) and Gold(I) Complexes of Aminofunctionalized Phosphinines: Synthesis and Structural Characterization" @default.
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- W4311361715 doi "https://doi.org/10.1002/zaac.202200365" @default.
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