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- W4311367443 abstract "Dynamic emissive materials in aqueous media have received much attention owing to their ease of preparation, tunable luminescence and environmental friendliness. However, hydrophobic fluorophores usually suffer from aggregation-caused quenching in water. In this work, we constructed an artificial light-harvesting system by using a non-covalent aggregation-induced emission dimer as antenna and energy donor. The dimer is quadruple hydrogen bonded from a ureidopyrimidinone derivative (M) containing a tetraphenylethylene group. The dispersed nano-assemblies based on the dimer in aqueous media were fabricated with the help of surfactant. By loading a hydrophobic acceptor molecule DBT into the nano-assemblies, man-made light-harvesting nanoparticles were fabricated, showing considerable energy transfer efficiency and a relatively high antenna effect. Additionally, the fluorescence color of the system can be gradually tuned by varying the content of the acceptors. This study provides a general way for the construction of an aqueous light-harvesting system based on a supramolecular dimer, which is important for potential application in luminescent materials." @default.
- W4311367443 created "2022-12-25" @default.
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- W4311367443 date "2022-12-14" @default.
- W4311367443 modified "2023-09-25" @default.
- W4311367443 title "Non-Covalent Dimer as Donor Chromophore for Constructing Artificial Light-Harvesting System in Water" @default.
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- W4311367443 doi "https://doi.org/10.3390/molecules27248876" @default.
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