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- W4311433025 abstract "The nonradiative carrier recombination at the perovskite/carrier selective layer (CSL) interface was accounted for the inferior power conversion efficiency (PCE) of perovskite solar cells (PSCs), especially rigid all-inorganic perovskite (CsPbI3 and CsPbBr3). In this study, targeting the poor interface, we introduce SbX3 (X = Cl, Br, I) surface passivation at the CsPbBr3/carbon interface. Smoothed compressive strain, reduced defect density, and enhanced energy-level alignment were achieved simultaneously, facilitating carrier extraction at the selective interface. With the simple aqueous solution-based two-step process, the PCE of our SbI3 passivated carbon-based CsPbBr3 PSCs has increased from 7.81% (without passivation) to 9.69%, a ∼25% enhancement. Specifically, Voc (1.657 V) of the SbI3-passivated cells was much higher than that of the control ones (1.488 V), confirming the ameliorated interface. Finally, our unencapsulated SbI3 passivated devices maintain 90% of their initial PCEs while left in the air for 30 days with a relative humidity of 60%. To conclude, we present an interfacial carrier extraction-enhanced strategy for preparing high-performance and stable CsPbBr3-based PSCs." @default.
- W4311433025 created "2022-12-26" @default.
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- W4311433025 date "2022-12-14" @default.
- W4311433025 modified "2023-10-16" @default.
- W4311433025 title "Facilitating the Carrier Transport Kinetics at the CsPbBr<sub>3</sub>/Carbon Interface through SbX<sub>3</sub> (X = Cl, Br, I) Passivation" @default.
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- W4311433025 doi "https://doi.org/10.1021/acsami.2c17046" @default.
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