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- W4311434067 abstract "The use of fully or partially absorbing boundary conditions for diffusion-based problems has become paradigmatic in physical chemistry and biochemistry to describe reactions occurring in solutions or in living media. However, as chemical states may indeed disappear, particles cannot, unless such degradation happens physically and should, thus, be accounted for explicitly. Here, we introduce a simple, yet general idea that allows one to derive the appropriate boundary conditions self-consistently from the chemical reaction scheme and the geometry of the physical reaction boundaries. As an illustration, we consider two paradigmatic examples, where the known results are recovered by taking specific physical limits. More generally, we demonstrate that our mathematical analysis delivers physical insight that cannot be accessed through standard treatments." @default.
- W4311434067 created "2022-12-26" @default.
- W4311434067 creator A5091096024 @default.
- W4311434067 date "2022-12-16" @default.
- W4311434067 modified "2023-09-24" @default.
- W4311434067 title "The physics of boundary conditions in reaction–diffusion problems" @default.
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- W4311434067 doi "https://doi.org/10.1063/5.0128276" @default.
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