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- W4311451736 abstract "We report a combined photoelectron spectroscopy and theoretical investigation of a series of size-selected hydrated closo-dodecaborate clusters B12X122-·nH2O (X = H, F, or I; n = 1-6). Distinct structural arrangements of water clusters from monomer to hexamer can be achieved by using different B12X122- bases, illustrating the evident solute specificity. Because B-H···H-O dihydrogen bonds are stronger than O···H-O hydrogen bonds in water, the added water molecules are arranged in a unified binding mode by forming highly structured water networks manipulated by B12H122-. As a comparison, the hydrated B12F122- clusters display similar water evolution for n values of 1 and 2 but different binding modes for larger clusters, while water networks in B12I122- share similarities with the free water clusters. This finding provides a consistent picture of the structural diversity of hydrogen bonding networks in microhydrated dodecaborates and a molecular-level understanding of microsolvation dynamics in aqueous borate chemistry." @default.
- W4311451736 created "2022-12-26" @default.
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- W4311451736 date "2022-12-14" @default.
- W4311451736 modified "2023-10-18" @default.
- W4311451736 title "Highly Structured Water Networks in Microhydrated Dodecaborate Clusters" @default.
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- W4311451736 doi "https://doi.org/10.1021/acs.jpclett.2c03537" @default.
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