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• W4311492054 endingPage "2212299" @default.
• W4311492054 startingPage "2212299" @default.
• W4311492054 abstract "High-performance rechargeable Zn-air batteries with long-life stability are desirable for power applications in electric vehicles. The key component of the Zn-air batteries is the bifunctional oxygen electrocatalyst, however, designing a bifunctional oxygen electrocatalyst with high intrinsic reversibility and durability is a challenge. Through density functional theory calculations, it is found that the catalytic activity originated from the electronic and geometric coordination structures synergistic effect of the Fe and Co dual-sites with metal-N4 coordination environment, assisting the stronger hybridization of electronic orbitals between Co (dxz, dz2) and OO* (px, pz), thus making the stronger O2 active ability of Co active site. These findings enable to development of a fancy dual single-atom catalyst comprising adjacent FeN4 and CoN4 sites on N-doped carbon matrix (FeCo-NC). FeCo-NC exhibits extraordinary bifunctional activities for oxygen reduction and evolution reaction (ORR/OER), which displays high half-wave potential (0.893 V) for the ORR, and low overpotential (343 mV) at 10 mA cm−2 for the OER. The assembled FeCo-NC air-electrode works well in the flexible solid-state Zn-air battery with a high specific capacity of 747.0 mAh g−1, a long-time stability of more than 400 h (30 °C), and also a superior performance at extreme temperatures (−30 °C–60 °C)." @default.
• W4311492054 created "2022-12-26" @default.
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• W4311492054 date "2022-12-14" @default.
• W4311492054 modified "2023-09-30" @default.
• W4311492054 title "Dual‐Sites Coordination Engineering of Single Atom Catalysts for Full‐Temperature Adaptive Flexible Ultralong‐Life Solid‐State Zn−Air Batteries" @default.
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• W4311492054 doi "https://doi.org/10.1002/adfm.202212299" @default.
• W4311492054 hasPublicationYear "2022" @default.
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