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- W4311494575 abstract "The unsatisfactory cycling stability of Zn anode stemming from dendritic growth and side reactions has slowed the rapid development of aqueous Zn-ion batteries (AZIBs). Constructing a three-dimensional (3D) artificial interphase layer is an appealing solution since it could dictate Zn deposition at the interface. Here, the in situ growth of a Cu-based metal–organic framework (Cu-MOF) over commercial Zn foil followed by subsequent selenization endows selenized Cu-MOF (SCM) with a stabilized Zn anode. The 3D SCM coating could homogenize the electric field and function as a reservoir to tolerate the deposited Zn. As a result, both rampant dendritic propagation and the notorious side reactions are concurrently inhibited. The SCM@Zn symmetric cell displays an elongated cyclic life for over 500 h at 2.0 mA cm–2. The assembled AZIB full cell readily realizes high electrochemical reversibility under different current densities. Our investigation offers insights into the design of a protective layer for high-performance Zn anodes." @default.
- W4311494575 created "2022-12-26" @default.
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- W4311494575 date "2022-12-14" @default.
- W4311494575 modified "2023-09-27" @default.
- W4311494575 title "Highly Stable Zn Anodes Modulated by Selenizing In Situ Grown Metal–Organic Frameworks" @default.
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- W4311494575 doi "https://doi.org/10.1021/acs.jpcc.2c07850" @default.
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