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- W4311597391 abstract "Together they solved the cold case! Activation of the distal C-H bonds of ferrocene and its stereoselective functionalization is not a dream anymore. Here we report, regio-and stereo selective catalytic distal C-H functionalization of ferrocenes actualizing the synthesis of ferrocene-1,3-derivatives by a Catellani-type reaction. The winning Pd/norbornene catalyst combination is able to reach hitherto inaccessible reaction site of ferrocene and accomplishes the regio-and stereoselective arylation of ferrocenylmethylamine. The ligand controlled synergistic Pd/norbornene metal-organic cooperative catalysis under aerobic conditions successfully achieves the synthesis of 30 ferrocene-1,3 derivatives in moderate to good yields and with high enantioselectivity in the substrates scanned." @default.
- W4311597391 created "2022-12-27" @default.
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- W4311597391 date "2022-12-16" @default.
- W4311597391 modified "2023-10-15" @default.
- W4311597391 title "The winning team reached the terra incognita: Enantioselective synthesis of ferrocene 1,3-derivatives via distal C-H activation by Pd(II)/norbornene cooperative catalysis" @default.
- W4311597391 doi "https://doi.org/10.26434/chemrxiv-2022-zc2vv" @default.
- W4311597391 hasPublicationYear "2022" @default.
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