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- W4311679046 abstract "In this work, we found that the presence of non-active ZnO crystals greatly accelerated the degradation of Bisphenol A (BPA) by 3.7 folds in the peroxymonosulfate (PMS, HSO5-)/Co3O4 system. Our mechanistic study revealed that the ZnO particles would create negative electric microfields around them, which are closely related with the zeta potentials (ζ) of ZnO and affected by solution pH. According to COMSOL simulation, the electrostatic repulsion between ZnO and PMS would drive HSO5- toward active Co3O4 surface, leading to the concentration increasing of HSO5- around active Co3O4 particles, which will then improve the degradation performance. The particle size of ZnO will also affect the promoting effect greatly by COMSOL simulation. Therefore, this study for the first time reveals synergy of electric microfields for enhanced heterogeneous Fenton-like reactions, providing a low-cost and effective strategy for enhanced persulfate catalysis." @default.
- W4311679046 created "2022-12-28" @default.
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- W4311679046 date "2023-03-01" @default.
- W4311679046 modified "2023-09-27" @default.
- W4311679046 title "Facilely achieved enhancement of Fenton-like reactions by constructing electric microfields" @default.
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- W4311679046 doi "https://doi.org/10.1016/j.jcis.2022.12.012" @default.
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