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- W4311703352 abstract "Aqueous redox flow batteries (ARFBs) exhibit great potential for large-scale energy storage, but the cross-contamination, limited ion conductivity, and high costs of ion-exchange membranes restrict the wide application of ARFBs. Herein, we report the construction of aqueous colloid flow batteries (ACFBs) based on redox-active polyoxometalate (POM) colloid electrolytes and size-exclusive membrane separators. The aqueous suspensions of POM clusters, such as [N(C3H7)4]4[H12(VO2)12(C6H5PO3)8]·xH2O and [N(C3H7)4]4[H12(VO2)12(4-FC6H4PO3)8]·xH2O, deliver good reversibility, high redox kinetics, and long cycling life. The nanoscale sizes of POM clusters make them compatible with cheap commercial dialysis membrane separators to replace expensive ion-exchange membranes, thus inhibiting the cross-contamination of active species via size exclusion. The ACFBs achieve a high energy efficiency of ∼90% and an ultralow capacity fade rate of 0.004% per cycle. This work highlights the great potential of ACFBs based on redox-reversible POM clusters and size-exclusion membrane separators toward grid-scale and sustainable energy storage applications." @default.
- W4311703352 created "2022-12-28" @default.
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- W4311703352 date "2022-12-06" @default.
- W4311703352 modified "2023-10-15" @default.
- W4311703352 title "Aqueous Colloid Flow Batteries Based on Redox-Reversible Polyoxometalate Clusters and Size-Exclusive Membranes" @default.
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- W4311703352 doi "https://doi.org/10.1021/acsenergylett.2c02121" @default.
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