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• W4311707465 abstract "The experimental fine and hyperfine structures of low npπ3Πu Rydberg states with n=2–4 measured in the 1970's for various vibration-rotation levels by Lichten and collaborators, and by Miller and Freund, are reanalysed in the framework of molecular frame-transformation multichannel quantum defect theory MQDT. Instead of the level by level treatment in terms of an effective Hamiltonian as was carried out at the time, a global theory is applied to all levels at once. It is found that the essence of the observed level patterns is well represented by MQDT in terms of a substantially reduced number of dynamical parameters – quantum defects – although the experimental accuracy of the experiments is not yet quite reached. Possible reasons for the remaining discrepancies are given. Since quantum defect theory MQDT, a formalism derived from scattering theory, is still rather little used in the domain of modern ultra-high precision spectroscopy, the occasion is taken here to review some of its key elements." @default.
• W4311707465 created "2022-12-28" @default.
• W4311707465 creator A5020330910 @default.
• W4311707465 date "2022-12-06" @default.
• W4311707465 modified "2023-09-30" @default.
• W4311707465 title "The fine and hyperfine structures of the low-<i>n</i> ³Π_<i>u</i> Rydberg states of H₂ revisited" @default.
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• W4311707465 doi "https://doi.org/10.1080/00268976.2022.2152396" @default.
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