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- W4311751509 abstract "Iron-based metal-organic frameworks are popular in the field of photocatalysis for their excellent visible light responsiveness. However, the rapid recombination of hole-electron pairs always limits its application. In this paper, a poly-nitrogen conjugated molecule, 1,1,2,2-Tetrakis(4-(pyridin-4-yl) phenyl) ethylene (TPPE) was simply modified on the surface of MIL-101(Fe) by alcohol-thermal method to tune its photocatalysis properties, and a novel nitrogenous core-shell MIL-101(Fe)-based nanocomposite (MIL-101(Fe)@TPPE) was prepared. The results showed that the hybrid material had a higher electron-hole separation rate and lower bandgap energy, along with a faster and stronger response to visible light compared with pure MIL-101(Fe). Batch studies showed that the optimized nanocomposite (MT-5) could efficiently photo-degrade TC, and the total removal rate was up to about 95% under visible light at pH 6 Additionally, MT-5 had very high adsorption capacity for tetracycline hydrochloride (TC), and the maximum adsorption capacity could reach 576.13 mg∙g−1. The studies on degradation mechanism proved that h+ and O2- played an important role during the photodegradation process. The degradation intermediates were analyzed, and QSAR was employed to evaluate the toxicity of TC and the intermediates. Furthermore, MT-5 exhibited good cycle stability, practical application, and environmental friendliness, which indicates its excellent applicable potential for organic pollutants removal." @default.
- W4311751509 created "2022-12-28" @default.
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- W4311751509 date "2023-03-01" @default.
- W4311751509 modified "2023-10-01" @default.
- W4311751509 title "A novel nitrogenous core-shell MIL-101(Fe)-based nanocomposite for enhanced adsorption and photo-degradation of organic pollutant under visible light" @default.
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- W4311751509 doi "https://doi.org/10.1016/j.jallcom.2022.168479" @default.
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