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• W4311752163 startingPage "112148" @default.
• W4311752163 abstract "One of the features of perovskite solar cells (PSCs) that make them stand out among all photovoltaics (PVs) is their high open-circuit voltage (VOC). Owing to their simple manufacturing process, low cost of components, and good stability, carbon electrode-based metal-halide PSCs are gaining interest for their better stability and low cost than noble metal electrodes. However, carbon electrode-based hybrid PSCs suffer low open-circuit voltage (VOC). This work demonstrated the fabrication of ambient processed hybrid perovskite solar cells using low-temperature curable carbon-based electrodes without a hole transport layer. The devices exhibit an impressive high open circuit voltage of 1.07 V, even without a dedicated hole transport layer. The photovoltaic performance was further investigated with the same perovskite absorber, synthesized by solution-processed and solid-state synthesis routes. The latter have yielded better short circuit current and power conversion efficiency due to perovskite's lesser built-in trap density. Furthermore, using a combined ionic electronic carrier transport model, an electric double-layer formation was ensured across the perovskite/carbon interface and accumulating halide vacancies at the perovskite/TiO2 interface can effectively reduce carrier recombination and boost the device's VOC. This study envisages the impact of the electric double layer in free carrier transport of an ionic-electronic semiconductor like hybrid perovskites and can pave the way to improve the open-circuit voltage of carbon-based perovskite solar cells." @default.
• W4311752163 created "2022-12-28" @default.
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• W4311752163 date "2023-03-01" @default.
• W4311752163 modified "2023-10-18" @default.
• W4311752163 title "Achieving high open circuit voltage for hole transport layer free ambient perovskite solar cells utilizing electric double layer effect" @default.
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• W4311752163 doi "https://doi.org/10.1016/j.solmat.2022.112148" @default.
• W4311752163 hasPublicationYear "2023" @default.
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