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• W4311763311 endingPage "11843" @default.
• W4311763311 startingPage "11837" @default.
• W4311763311 abstract "Although seeking an effective strategy for further improving their optical properties is a great challenge, two-dimensional (2D) halide perovskites have attracted a significant amount of attention because of their performance. In this regard, the pressure-induced emission accompanied by a remarkable pressure-enhanced emission is achieved without a phase transition in 2D vacancy-ordered perovskite Cs3Bi2Cl9 nanocrystals (NCs). Note that the initial Cs3Bi2Cl9 NCs possess extremely strong electron-phonon coupling, leading to the easy annihilation of trapped excitons by the phonon. Upon compression, pressure could effectively suppress phonon-assisted nonradiative decay and give rise to an intriguing emission from 0 to 1. Both the weakened electron-phonon coupling and the relaxed halide octahedral distortion benefiting from the vacancy-ordered structure contributed to the subsequent enhanced emission. This work not only elucidates the underlying photophysical mechanism but also identifies pressure engineering as a robust means for improving their potential applications in environmentally friendly solid-state lighting at extremes." @default.
• W4311763311 created "2022-12-28" @default.
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• W4311763311 date "2022-12-15" @default.
• W4311763311 modified "2023-10-14" @default.
• W4311763311 title "Pressure-Induced Emission from All-Inorganic Two-Dimensional Vacancy-Ordered Lead-Free Metal Halide Perovskite Nanocrystals" @default.
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• W4311763311 doi "https://doi.org/10.1021/acs.jpclett.2c03332" @default.
• W4311763311 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36520022" @default.
• W4311763311 hasPublicationYear "2022" @default.
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