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• W4311773304 abstract "Abstract Electrochemical CO 2 reduction is an environmentally sustainable way for CO 2 conversion and utilization, the development of which needs highly efficient catalysts. Ag‐based materials are one kind of electrocatalyst that are catalytically active for CO 2 reduction to CO. In this work, Ag clusters were fabricated on nitrogen‐doped porous carbon nanomaterials by a high‐temperature annealing method. The well‐dispersion of Ag sites on nitrogen‐doped carbons (Ag/NC) promoted CO production. As a result, Ag/NC showed a maximum Faradaic efficiency of 94 % at −0.7 V versus reversible hydrogen electrode (vs RHE) at room temperature. In addition, Ag/NC showed good CO 2 reduction stability, and the CO Faradaic efficiency remained stable at about 90 % at −0.7 V vs RHE for 12 h. Density functional theory calculation indicated that the cooperation of Ag and N‐dopings effectively reduced the activation energy barrier of CO 2 reduction relative to hydrogen evolution reaction and thus effectively promoted the electrocatalytic reduction of CO 2 molecules to CO. This method provides a new idea for the synthesis of CO 2 reduction catalysts with higher activity, selectivity and stability." @default.
• W4311773304 created "2022-12-28" @default.
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• W4311773304 date "2022-12-15" @default.
• W4311773304 modified "2023-10-15" @default.
• W4311773304 title "Nitrogen Defects in Porous Carbons with Adjacent Silver Nanoclusters for Efficient CO₂ Reduction" @default.
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• W4311773304 doi "https://doi.org/10.1002/celc.202200987" @default.
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