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• W4311781710 abstract "Single-atom catalysts offer a promising pathway for electrochemical CO2 conversion. However, it is still a challenge to optimize the electrochemical performance of dual-atom catalysts. Here, an atomic indium-nickel dual-sites catalyst bridged by an axial oxygen atom (O-In-N6-Ni moiety) was anchored on nitrogenated carbon (InNi DS/NC). InNi DS/NC exhibits superior CO selectivity with Faradaic efficiency higher than 90 % over a wide potential range from −0.5 to −0.8 V versus reversible hydrogen electrode (vs. RHE). Moreover, an industrial CO partial current density up to 317.2 mA cm−2 is achieved at −1.0 V vs. RHE in a flow cell. In situ ATR-SEIRAS combined with theory calculations reveal that the synergistic effect of In-Ni dual-sites and O atom bridge not only reduces the reaction barrier for the formation of *COOH, but also retards the undesired hydrogen evolution reaction. This work provides a feasible strategy to construct dual-site catalysts towards energy conversion." @default.
• W4311781710 created "2022-12-28" @default.
• W4311781710 creator A5003237621 @default.
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• W4311781710 creator A5081131905 @default.
• W4311781710 creator A5081566869 @default.
• W4311781710 date "2023-01-11" @default.
• W4311781710 modified "2023-10-05" @default.
• W4311781710 title "Oxygen‐Bridged Indium‐Nickel Atomic Pair as Dual‐Metal Active Sites Enabling Synergistic Electrocatalytic CO₂ Reduction" @default.
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• W4311781710 doi "https://doi.org/10.1002/ange.202216326" @default.
• W4311781710 hasPublicationYear "2023" @default.
• W4311781710 type Work @default.
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