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- W4311843119 abstract "Understanding the effects of halogens on the production of macromolecular disinfection byproducts (DBPs) is critical for drinking water safety. The effects of Br- and I- on the chemical diversity of dissolved organic matter (DOM) during plasma preoxidation and the subsequent formation of macromolecular halogenated DBPs after chlorination were deciphered. Plasma preoxidation changed DOM diversity from aromatic component-oriented to lignin and tannin component-oriented, resulting in 62.0% and 21.2% decreases in N-DBPs (CkHnOmNzClx formulas) and C-DBPs (CkHnOmClx formulas) after chlorination, respectively. Br- could induce the formation of organobromine compounds (OBrCs) during plasma oxidation; however, the intensities of OBrCs decreased by 56.3% (CHO formulas) and 75.2% (CHON formulas) after further chlorination. OBrCs still accounted for 79.8% of the total organohalogen compounds (OXCs, X=Cl or Br) due to the higher substitutability of bromine. I-promoted OIC production in the DOM preoxidation process, and OICs acted as intermediates to form OClCs during chlorination. When Br-and I-coexisted, Br- promoted OIC production in the DOM preoxidation process; therefore, more OBrCs and OClCs were generated due to intermediates of OICs in subsequent chlorination. Connections between OXCs and their precursors were established using network computation. The precursors of OClCs were located in the aromatic structure region (0.2 < H/C ≤ 0.7; O/C ≤ 0.67); those of OBrCs and OICs were located in the lignin (0.7 < H/C ≤ 1.5; 0.1 < O/C < 0.67) and tannin (0.6 ≤ H/C ≤ 1.5, 0.67 < O/C < 1.0) regions with relatively greater H/C and O/C ratios, respectively." @default.
- W4311843119 created "2023-01-01" @default.
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- W4311843119 date "2023-02-01" @default.
- W4311843119 modified "2023-10-17" @default.
- W4311843119 title "Formation of halogenated macromolecular organics induced by Br− and I− during plasma oxidation/chlorination of DOM: Highlighting competitive mechanisms" @default.
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- W4311843119 doi "https://doi.org/10.1016/j.watres.2022.119513" @default.
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