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• W4311941007 abstract "The study of optical transitions in lanthanide(III) ions has evolved separately from molecular photophysics, but the framework still applies to these forbidden transitions. In this study, a detailed photophysical characterization of the [Tb(H2O)9]3+ aqua ion was performed. The luminescence quantum yield (Φlum), excited state lifetime (τobs), radiative (kr ≡ A) and nonradiative (knr) rate constants, and oscillator strength (f) were determined for Tb(CF3SO3)3 in H2O/D2O mixtures in order to map the radiative and nonradiative transition probabilities. It was shown that the intense luminescence observed from Tb3+ compared to other Ln3+ ions is not due to a higher transition probability of emission but rather due to a lack of quenching, quantified by quenching to O-H oscillators in the aqua ion of kq(OH) = 2090 s-1 for terbium and kq(OH) = 8840 s-1 for europium. In addition, the Horrocks method of determining inner-sphere solvent molecules has been revisited, and it was concluded that the Tb3+ is 9-coordinated in aqueous solution." @default.
• W4311941007 created "2023-01-02" @default.
• W4311941007 creator A5056546144 @default.
• W4311941007 creator A5074462988 @default.
• W4311941007 date "2022-12-19" @default.
• W4311941007 modified "2023-09-29" @default.
• W4311941007 title "Tb³⁺ Photophysics: Mapping Excited State Dynamics of [Tb(H₂O)₉]³⁺ Using Molecular Photophysics" @default.
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• W4311941007 doi "https://doi.org/10.1021/acs.jpclett.2c03506" @default.
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