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- W4312010651 abstract "Hydrodynamic interactions (HIs) play a critical role in the self-organization of colloidal suspensions and biological solutions. However, their roles have remained elusive particularly for charged soft matter systems. Here we consider the role of HIs in the self-assembly of oppositely charged colloidal particles, which is a promising candidate for electrical tunable soft materials. We employ the fluid particle dynamics method to consider many-body HIs and the coupling between the colloid, ion, and fluid motions. We find that, under a constant electric field, oppositely charged colloidal particles form clusters and percolate into a gel network, unlike bundlelike aggregates aligned in the field direction observed by Brownian dynamics simulations neglecting HIs. We reveal that the cluster-forming tendency originates from the incompressibility-induced inverse squeezing flow effect that dramatically slows down the disaggregation of attached colloids. Our findings indicate that the HI selects a unique kinetic pathway to the nonequilibrium colloidal self-assembly." @default.
- W4312010651 created "2023-01-03" @default.
- W4312010651 creator A5005967783 @default.
- W4312010651 creator A5069127789 @default.
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- W4312010651 date "2022-12-09" @default.
- W4312010651 modified "2023-10-16" @default.
- W4312010651 title "Impact of Inverse Squeezing Flow on the Self-Assembly of Oppositely Charged Colloidal Particles under Electric Field" @default.
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- W4312010651 doi "https://doi.org/10.1103/physrevlett.129.248001" @default.
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