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- W4312085110 endingPage "122297" @default.
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- W4312085110 abstract "Developing rhodium-based electrocatalysts with strong metal-support interaction (SMSI) is crucial for hydrogen evolution reaction (HER) in full pH range, but it is still challenging. In this work, a boron doping strategy is proposed to activate the SMSI of ultra-small Rh nanoparticles encapsulated by N-doped carbon matrix ([email protected]). Density functional theory (DFT) reveals that boron doping can regulate the electronic structure and the water adsorption energy, further boosting the HER activity. Consequently, the as-prepared [email protected] nanospheres possess Pt-like activity for HER with low overpotentials in 1.0 M KOH (η10 = 26 mV), 0.5 M H2SO4 (η10 = 43 mV), and 1.0 M PBS (η10 = 70 mV), as well as outstanding stability. This work opens up a new way to construct remarkable pH-universal electrocatalysts." @default.
- W4312085110 created "2023-01-04" @default.
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- W4312085110 date "2023-05-01" @default.
- W4312085110 modified "2023-09-28" @default.
- W4312085110 title "Boron doping activate strong metal-support interaction for electrocatalytic hydrogen evolution reaction in full pH range" @default.
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- W4312085110 doi "https://doi.org/10.1016/j.apcatb.2022.122297" @default.
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