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- W4312095801 abstract "Stimuli-responsive opposite emission (A)/absorption (B) polymer material (A∪B = Ω and A∩B = Ø) represents a novel polymer material that is difficult to prepare. Here, we demonstrate a one-pot strategy for the molecular design of stimuli-responsive opposite emission/absorption polymer material with intriguing properties of opposite emission/absorption and aggregation-induced emission (AIE) type nontraditional intrinsic luminescence (NTIL) in the visible region, through reversible addition–fragmentation chain transfer polymerization-induced emission (PIE) of the N,N-dimethyl-triphenylmethanol moiety. Investigations reveal that NTIL is due to the through-space conjugation effect caused by polymer chain entanglement, when increasing the repeating unit number. The corresponding stimuli-responsive opposite emission/absorption properties are derived from the carbocation-quinoid mechanism, which enables the fluorescence encryption capability. This work therefore demonstrates the proof of concept of a novel opposite emission/absorption polymer material that might cause inspiration in different fields." @default.
- W4312095801 created "2023-01-04" @default.
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- W4312095801 date "2022-12-22" @default.
- W4312095801 modified "2023-10-02" @default.
- W4312095801 title "One-Pot Synthesis of Stimuli-Responsive Fluorescent Polymers through Polymerization-Induced Emission" @default.
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- W4312095801 doi "https://doi.org/10.1021/acsmacrolett.2c00653" @default.
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