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- W4312114827 abstract "Two-dimensional metal-organic frameworks (2D MOFs) can be used as the cathodes for high-performance zinc-ion battery due to their large one-dimensional channels. However, the conventionally poor electrical conductivity and low structural stability hinder their advances. Herein, we report an alternately stacked MOF/MX heterostructure, exhibiting the 2D sandwich-like structure with abundant active sites, improved electrical conductivity and exceptional structural stability. Ex situ characterizations and theoretical calculations reveal a reversible intercalation mechanism of zinc ions and high electrical conductivity in the 2D heterostructure. Electrochemical tests confirm excellent Zn2+ migration kinetics and ideal pseudocapacitive behaviors. As a consequence, Cu-HHTP/MX shows a superior rate performance (260.1 mAh g-1 at 0.1 A g-1 and 173.1 mAh g-1 at 4 A g-1 ) and long-term cycling stability of 92.5 % capacity retention over 1000 cycles at 4 A g-1 ." @default.
- W4312114827 created "2023-01-04" @default.
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- W4312114827 date "2023-01-18" @default.
- W4312114827 modified "2023-10-17" @default.
- W4312114827 title "Constructing 2D Sandwich‐like MOF/MXene Heterostructures for Durable and Fast Aqueous Zinc‐Ion Batteries" @default.
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- W4312114827 doi "https://doi.org/10.1002/anie.202218343" @default.
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