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- W4312118979 abstract "In aqueous zinc ion batteries (ZIBs), the H+ intercalation possesses superior electrochemical kinetics with excellent rate capability, however, precisely modulating H+ intercalation has been still challenging. Herein, a critical modification of pre-intercalating metal ions in the MnO2 interlayer (M−MnO2) with controllable p-band center (ϵp) of O is reported to modulate the H+ intercalation. The modulation of metal-O bond type and covalency degree on the average charge of O atom results in optimized ϵp and H+ adsorption energy for M−MnO2, thus promoting the balance between H+ adsorption and desorption, which plays a determinant role on H+ intercalation. The optimized Cu−MnO2 delivers superior rate capability with the capacity of 153 mAh g−1 at a high rate of 3 A g−1 after 1000 cycles. This work demonstrates that ϵp could be a significant descriptor for H+ intercalation, and tuning ϵp effectively increases H+ intercalation contribution with excellent rate capability in ZIBs." @default.
- W4312118979 created "2023-01-04" @default.
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- W4312118979 date "2023-01-18" @default.
- W4312118979 modified "2023-10-15" @default.
- W4312118979 title "Engineering p‐Band Center of Oxygen Boosting H <sup>+</sup> Intercalation in δ‐MnO <sub>2</sub> for Aqueous Zinc Ion Batteries" @default.
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- W4312118979 doi "https://doi.org/10.1002/ange.202215654" @default.
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