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- W4312164524 abstract "Abstract Electrochemically reducing CO 2 to valuable fuels or feedstocks is recognized as a promising strategy to simultaneously tackle the crises of fossil fuel shortage and carbon emission. Sn‐based catalysts have been widely studied for electrochemical CO 2 reduction reaction (CO 2 RR) to make formic acid/formate, which unfortunately still suffer from low activity, selectivity and stability. In this work, halogen (F, Cl, Br or I) was introduced into the Sn catalyst by a facile hydrolysis method. The presence of halogen was confirmed by a collection of ex situ and in situ characterizations, which rendered a more positive valence state of Sn in halogen‐incorporated Sn catalyst as compared to unmodified Sn under cathodic potentials in CO 2 RR and therefore tuned the adsorption strength of the key intermediate (*OCHO) toward formate formation. As a result, the halogen‐incorporated Sn catalyst exhibited greatly enhanced catalytic performance in electrochemical CO 2 RR to produce formate." @default.
- W4312164524 created "2023-01-04" @default.
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- W4312164524 date "2023-01-24" @default.
- W4312164524 modified "2023-10-14" @default.
- W4312164524 title "Halogen‐Incorporated Sn Catalysts for Selective Electrochemical CO<sub>2</sub> Reduction to Formate" @default.
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- W4312164524 doi "https://doi.org/10.1002/ange.202211174" @default.
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