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• W4312225686 abstract "The uncontrollable growth of lithium (Li) dendrites and the instability of the Li/electrolyte interface hinder the development of next-generation rechargeable lithium metal batteries. The combination of inorganic nanoparticles and polymers as the artificial SEI layer shows great potential in regulating lithium-ion flux. Here, we design spatially confined LiF nanoparticles in an aligned polymer matrix as the artificial SEI layer. A high dielectric polymer matrix homogenizes the electric field near the surface of lithium metal. Aligned pores with LiF nanoparticles promote the lithium-ion transport across the artificial SEI layer. The synergistic effect of the highly polar β-phase PVDF and LiF nanoparticles provides high stability over 900 h for the Li//Li symmetrical cell. Besides, a Li//LFP full battery equipped with this artificial layer shows good performance in the commercial carbonate electrolyte, demonstrating the great potential of this protective film in lithium metal batteries." @default.
• W4312225686 created "2023-01-04" @default.
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• W4312225686 date "2022-12-28" @default.
• W4312225686 modified "2023-10-17" @default.
• W4312225686 title "Spatially Confined LiF Nanoparticles in an Aligned Polymer Matrix as the Artificial SEI Layer for Lithium Metal Anodes" @default.
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• W4312225686 doi "https://doi.org/10.1021/acs.nanolett.2c04242" @default.
• W4312225686 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36576749" @default.
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