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- W4312387396 abstract "of these diagnostic techniques at 600 Torr (800 mbar) pressure and temperatures from 150 to 410 °C. Planar laser-induced fluorescence provides two-dimensional images of the formaldehyde product distribution that show the development of the boundary layer above the catalyst under different flow conditions. Raman scattering imaging provides measurements of a wide range of major species, such as methanol, oxygen, nitrogen, formaldehyde, and water vapor. Near-surface molecular beam mass spectrometry enables simultaneous detection of all species using a gas sampling probe. Detection of gas-phase free radicals, such as CH3 and CH3O, and of minor products, such as acetaldehyde, dimethyl ether, and methyl formate, provides insights into catalytic mechanisms of the partial oxidation of methanol. The combination of these techniques provides a detailed picture of the coupling between the gas phase and surface in heterogeneous catalysis and enables parametric studies under different operating conditions, which will enhance our ability to constrain microkinetic models of heterogeneous catalysis." @default.
- W4312387396 created "2023-01-04" @default.
- W4312387396 creator A5061785195 @default.
- W4312387396 date "2021-10-01" @default.
- W4312387396 modified "2023-09-27" @default.
- W4312387396 title "Imaging the Gas Phase above a Reacting Surface: Partial Oxidation of Methanol over a Silver Catalyst." @default.
- W4312387396 doi "https://doi.org/10.2172/1891738" @default.
- W4312387396 hasPublicationYear "2021" @default.
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