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- W4312792315 endingPage "2483" @default.
- W4312792315 startingPage "2453" @default.
- W4312792315 abstract "Single-atom catalysts (SACs) have been widely used in heterogeneous catalysis owing to the maximum utilization of metal-active sites with controlled structures and well-defined locations. Upon tailored coordination with nitrogen atom, the metal-nitrogen (M-N)-based SACs have demonstrated interesting physical, optical and electronic properties and have become intense in photocatalysis and electrocatalysis in the past decade. Despite substantial efforts in constructing various M–N-based SACs, the principles for modulating the intrinsic photocatalytic and electrocatalytic performance of their active sites and catalytic mechanism have not been sufficiently studied. Herein, the present review intends to shed some light on recent research made in studying the correlation between intrinsic electronic structure, catalytic mechanism, single-metal atom (SMA) confinement and their photocatalytic and electrocatalytic activities (conversion, selectivity, stability and etc). Based on the analysis of fundamentals of M–N-based SACs, theoretical calculations and experimental investigations, including synthetic methods and characterization techniques, are both included to provide an integral understanding of the underlying mechanisms behind improved coordination structure and observed activity. Finally, the challenges and perspectives for constructing highly active M–N based photocatalysis and electrocatalysis SACs are provided. In particular, extensive technical and mechanism aspects are thoroughly discussed, summarized and analyzed for promoting further advancement of M-N-based SACs in photocatalysis and electrocatalysis." @default.
- W4312792315 created "2023-01-05" @default.
- W4312792315 creator A5003079852 @default.
- W4312792315 creator A5008688981 @default.
- W4312792315 creator A5013787745 @default.
- W4312792315 creator A5018028838 @default.
- W4312792315 creator A5022526821 @default.
- W4312792315 creator A5029360035 @default.
- W4312792315 creator A5073592102 @default.
- W4312792315 date "2022-01-01" @default.
- W4312792315 modified "2023-10-15" @default.
- W4312792315 title "Heterogeneous N-coordinated single-atom photocatalysts and electrocatalysts" @default.
- W4312792315 cites W1853374276 @default.
- W4312792315 cites W1875376631 @default.
- W4312792315 cites W1968213181 @default.
- W4312792315 cites W1969252570 @default.
- W4312792315 cites W1970127494 @default.
- W4312792315 cites W1973967873 @default.
- W4312792315 cites W1979371521 @default.
- W4312792315 cites W1981626052 @default.
- W4312792315 cites W1993998340 @default.
- W4312792315 cites W2003726195 @default.
- W4312792315 cites W2023070783 @default.
- W4312792315 cites W2032100925 @default.
- W4312792315 cites W2042492216 @default.
- W4312792315 cites W2050852068 @default.
- W4312792315 cites W2062049711 @default.
- W4312792315 cites W2078626024 @default.
- W4312792315 cites W2081994669 @default.
- W4312792315 cites W2109694766 @default.
- W4312792315 cites W2134716155 @default.
- W4312792315 cites W2140236911 @default.
- W4312792315 cites W2147452015 @default.
- W4312792315 cites W2170456486 @default.
- W4312792315 cites W2181522365 @default.
- W4312792315 cites W2189000696 @default.
- W4312792315 cites W2224728609 @default.
- W4312792315 cites W2255007534 @default.
- W4312792315 cites W2269800614 @default.
- W4312792315 cites W2290645004 @default.
- W4312792315 cites W2298579473 @default.
- W4312792315 cites W2298894995 @default.
- W4312792315 cites W2302371264 @default.
- W4312792315 cites W2312413687 @default.
- W4312792315 cites W2320849513 @default.
- W4312792315 cites W2326170978 @default.
- W4312792315 cites W2326928258 @default.
- W4312792315 cites W2340423559 @default.
- W4312792315 cites W2343203850 @default.
- W4312792315 cites W2345936754 @default.
- W4312792315 cites W2406103201 @default.
- W4312792315 cites W2432332453 @default.
- W4312792315 cites W2474207091 @default.
- W4312792315 cites W2474398724 @default.
- W4312792315 cites W2496132953 @default.
- W4312792315 cites W2502288548 @default.
- W4312792315 cites W2514233284 @default.
- W4312792315 cites W2531551506 @default.
- W4312792315 cites W2531629454 @default.
- W4312792315 cites W2536246483 @default.
- W4312792315 cites W2542763126 @default.
- W4312792315 cites W2557861838 @default.
- W4312792315 cites W2575823937 @default.
- W4312792315 cites W2591446277 @default.
- W4312792315 cites W2603037843 @default.
- W4312792315 cites W2605515801 @default.
- W4312792315 cites W2607231338 @default.
- W4312792315 cites W2617194355 @default.
- W4312792315 cites W2620180261 @default.
- W4312792315 cites W2734196657 @default.
- W4312792315 cites W2735002352 @default.
- W4312792315 cites W2736999751 @default.
- W4312792315 cites W2742542637 @default.
- W4312792315 cites W2749211685 @default.
- W4312792315 cites W2755768317 @default.
- W4312792315 cites W2761150275 @default.
- W4312792315 cites W2761427375 @default.
- W4312792315 cites W2765652562 @default.
- W4312792315 cites W2767180447 @default.
- W4312792315 cites W2767948854 @default.
- W4312792315 cites W2768067603 @default.
- W4312792315 cites W2770355995 @default.
- W4312792315 cites W2770634528 @default.
- W4312792315 cites W2773935583 @default.
- W4312792315 cites W2775347347 @default.
- W4312792315 cites W2776687276 @default.
- W4312792315 cites W2778748326 @default.
- W4312792315 cites W2781485885 @default.
- W4312792315 cites W2783027847 @default.
- W4312792315 cites W2784943348 @default.
- W4312792315 cites W2785307491 @default.
- W4312792315 cites W2786709116 @default.
- W4312792315 cites W2787298764 @default.
- W4312792315 cites W2789745531 @default.
- W4312792315 cites W2789860986 @default.
- W4312792315 cites W2790507915 @default.
- W4312792315 cites W2791476032 @default.
- W4312792315 cites W2793353452 @default.