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- W4313200118 abstract "Al-based composites for hydrogen generation possess many advantages like relatively high H2 capacity and low cost, but their application is hindered by the easy formation of alumina membrane on the Al surface. In this work, a novel flower-like [email protected] composite has been fabricated firstly, and then introduced into Al powders by ball milling (Al–[email protected]powder) or ball milling combining spark plasma sintering (SPS) (Al–[email protected]block). It is found that the flower-like [email protected] can significantly promote the H2 generation from Al-water reactions. Moreover, the performance of Al–[email protected]powder for H2 generation can be further improved by SPS treatment. The Al-7 wt% [email protected]block exhibits excellent H2 release performance at room temperature with a H2 yield of 1172.9 mL·g−1 and a conversion yield of 92.7% compared with Al-7 wt% [email protected]powder (864.9 mL·g−1 and 68.4%). Furthermore, the Al–[email protected]block demonstrates a favorable oxidation resistance, such as a H2 yield of 912.5 mL·g−1 even after being exposed to air for 35 days. The X-ray diffraction (XRD) analysis illustrates the formation of Bi, Bi2O3 and AlCl3 in situ can enhance the Al-water reaction. Density functional theory calculation reveals doped Bi or Bi2O3 can promote charges transfer from Al to Bi or Bi2O3. And the doped Bi can enhance the adsorption of H2O on the Al surface to improve H2 generation of the Al–[email protected]" @default.
- W4313200118 created "2023-01-06" @default.
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- W4313200118 date "2023-03-01" @default.
- W4313200118 modified "2023-09-26" @default.
- W4313200118 title "Enhanced hydrogen generation performances and mechanism of Al-water reaction catalyzed by flower-like BiOCl@CNTs" @default.
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- W4313200118 doi "https://doi.org/10.1016/j.mtnano.2022.100300" @default.
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