Matches in SemOpenAlex for { <https://semopenalex.org/work/W4313201390> ?p ?o ?g. }
- W4313201390 endingPage "140910" @default.
- W4313201390 startingPage "140910" @default.
- W4313201390 abstract "Efficient electrocatalytic conversion of CO2 to CO is a promising mode for CO2 transformation driven by renewable electricity. Herein, varied poly(ionic liquid)-Ag (PIL-Ag) hybrids are facilely synthesized by impregnating chloride-based PIL with silver salts. The remarkable confinement effect of PIL on the patterns of in-situ formed highly dispersed Ag–Cl species leads to the corresponding complexes, clusters, and nanoparticles (NPs) in the inner domain, while their distribution is highly correlated to both microstructures of the PIL skeleton and silver salts launched. As a result, the highly dispersed imidazolium-pyridine-imidazolium tridentate sites at the PIL layer combined with a compatible supply rate of Ag+ cation enables the formation of abundant AgCl NPs in [email protected], which provided a high CO selectivity of 96.8 % with a high partial current density of 207.0 mA cm−2 at –0.91 V (vs RHE) in 1 M KOH. Besides, long-term electrolysis was conducted at 100 mA cm−2 for 100 h with a slight decay of selectivity to ∼ 86 %. Further, despite the similar intrinsic activity of three Ag–Cl species, the patterns of Ag–Cl species, the number of active sites, and the mass transfer of reactants within the hybrids jointly determine the apparent electrocatalytic performance obtained at high rates." @default.
- W4313201390 created "2023-01-06" @default.
- W4313201390 creator A5014335750 @default.
- W4313201390 creator A5054207319 @default.
- W4313201390 creator A5062872235 @default.
- W4313201390 creator A5075289755 @default.
- W4313201390 date "2023-01-01" @default.
- W4313201390 modified "2023-09-23" @default.
- W4313201390 title "Efficient electrocatalytic reduction of CO2 to CO on highly dispersed Ag nanoparticles confined by Poly(ionic liquid)" @default.
- W4313201390 cites W1975798107 @default.
- W4313201390 cites W1978171666 @default.
- W4313201390 cites W1980103433 @default.
- W4313201390 cites W2002881973 @default.
- W4313201390 cites W2011851250 @default.
- W4313201390 cites W2014464559 @default.
- W4313201390 cites W2015536795 @default.
- W4313201390 cites W2028266484 @default.
- W4313201390 cites W2035709543 @default.
- W4313201390 cites W2062160443 @default.
- W4313201390 cites W2072505846 @default.
- W4313201390 cites W2103622038 @default.
- W4313201390 cites W2315123348 @default.
- W4313201390 cites W2323513112 @default.
- W4313201390 cites W2327255253 @default.
- W4313201390 cites W2509206142 @default.
- W4313201390 cites W2560046959 @default.
- W4313201390 cites W2624172309 @default.
- W4313201390 cites W2725074710 @default.
- W4313201390 cites W2761941514 @default.
- W4313201390 cites W2783311359 @default.
- W4313201390 cites W2788219036 @default.
- W4313201390 cites W2790006205 @default.
- W4313201390 cites W2800305228 @default.
- W4313201390 cites W2810755092 @default.
- W4313201390 cites W2884802060 @default.
- W4313201390 cites W2891376110 @default.
- W4313201390 cites W2892330472 @default.
- W4313201390 cites W2901156234 @default.
- W4313201390 cites W2965092797 @default.
- W4313201390 cites W2972593701 @default.
- W4313201390 cites W3004850479 @default.
- W4313201390 cites W3047670264 @default.
- W4313201390 cites W3112294465 @default.
- W4313201390 cites W3122837940 @default.
- W4313201390 cites W3125648545 @default.
- W4313201390 cites W3135651892 @default.
- W4313201390 cites W3142018483 @default.
- W4313201390 cites W3159808476 @default.
- W4313201390 cites W3162876756 @default.
- W4313201390 cites W3176782386 @default.
- W4313201390 cites W3198288772 @default.
- W4313201390 cites W3217709238 @default.
- W4313201390 cites W4206162368 @default.
- W4313201390 cites W4225270704 @default.
- W4313201390 cites W4240112750 @default.
- W4313201390 cites W4281976569 @default.
- W4313201390 cites W4283799034 @default.
- W4313201390 cites W4285591856 @default.
- W4313201390 cites W4308493215 @default.
- W4313201390 doi "https://doi.org/10.1016/j.cej.2022.140910" @default.
- W4313201390 hasPublicationYear "2023" @default.
- W4313201390 type Work @default.
- W4313201390 citedByCount "2" @default.
- W4313201390 countsByYear W43132013902023 @default.
- W4313201390 crossrefType "journal-article" @default.
- W4313201390 hasAuthorship W4313201390A5014335750 @default.
- W4313201390 hasAuthorship W4313201390A5054207319 @default.
- W4313201390 hasAuthorship W4313201390A5062872235 @default.
- W4313201390 hasAuthorship W4313201390A5075289755 @default.
- W4313201390 hasConcept C118792377 @default.
- W4313201390 hasConcept C127413603 @default.
- W4313201390 hasConcept C147789679 @default.
- W4313201390 hasConcept C154881586 @default.
- W4313201390 hasConcept C155672457 @default.
- W4313201390 hasConcept C161790260 @default.
- W4313201390 hasConcept C163127949 @default.
- W4313201390 hasConcept C171250308 @default.
- W4313201390 hasConcept C17525397 @default.
- W4313201390 hasConcept C178790620 @default.
- W4313201390 hasConcept C179104552 @default.
- W4313201390 hasConcept C185592680 @default.
- W4313201390 hasConcept C192562407 @default.
- W4313201390 hasConcept C2778695967 @default.
- W4313201390 hasConcept C2779485729 @default.
- W4313201390 hasConcept C42360764 @default.
- W4313201390 hasConcept C68801617 @default.
- W4313201390 hasConceptScore W4313201390C118792377 @default.
- W4313201390 hasConceptScore W4313201390C127413603 @default.
- W4313201390 hasConceptScore W4313201390C147789679 @default.
- W4313201390 hasConceptScore W4313201390C154881586 @default.
- W4313201390 hasConceptScore W4313201390C155672457 @default.
- W4313201390 hasConceptScore W4313201390C161790260 @default.
- W4313201390 hasConceptScore W4313201390C163127949 @default.
- W4313201390 hasConceptScore W4313201390C171250308 @default.
- W4313201390 hasConceptScore W4313201390C17525397 @default.
- W4313201390 hasConceptScore W4313201390C178790620 @default.
- W4313201390 hasConceptScore W4313201390C179104552 @default.
- W4313201390 hasConceptScore W4313201390C185592680 @default.