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- W4313201767 abstract "Herein, a novel deep eutectic solvent (DES) as suitable electrolyte is prepared by means of ethylene glycol (EG) and tetra methyl ammonium chloride (TMAC), and seven amino acids with different acidities are used as additives to explore the effect of amino acid on the voltage window of the electrolyte. The prepared serial DES are systematic studied and used as the electrolytes in supercapacitor. The results show that the addition of basic amino acids significantly increase the voltage window of the prepared DES electrolyte, neutral amino acids slightly increase the voltage window, and the acidic amino acids reduce the voltage window of the electrolyte. The proposed mechanism is that basic amino acids preferentially adsorb on the electrode surface increases the distance between chloride ions and the interface, thus hindering the oxidation of chloride ions. The high conductivity (3.51 mS cm−1) and low viscosity (30.4 cP) of DES electrolyte formed by EG, TMAC and arginine (Arg) is well suited in supercapacitors. Comparing with the electrolyte of non amino acids additive, using the optimized TMAC-EG-Arg-1.2 as electrolyte, the voltage window of the assembled activated carbon based supercapacitor is increased from 0.9 V to 2.0 V, and the energy density is as high as 20.55 Wh kg−1. Furthermore, the electrolyte has a wide operating temperature range (−20 ∼ 100 °C). This study uncovers a new possibility for enlarging the voltage window of DES electrolyte by addition of amino acids, which used as electrolyte with high performance in supercapacitor." @default.
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- W4313201767 date "2023-02-01" @default.
- W4313201767 modified "2023-10-10" @default.
- W4313201767 title "Amino acids assisted to improve the voltage window of deep eutectic electrolyte formed by ethylene glycol and tetra methyl ammonium chloride" @default.
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- W4313201767 doi "https://doi.org/10.1016/j.cej.2022.141143" @default.
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