Matches in SemOpenAlex for { <https://semopenalex.org/work/W4313201817> ?p ?o ?g. }
- W4313201817 endingPage "140721" @default.
- W4313201817 startingPage "140721" @default.
- W4313201817 abstract "Precise synthesis of single-atom catalysts (SACs) with both high loading and special configuration, not just transition metal-nitrogen co-doped carbon (M−Nx−C), to achieve large-scale and widespread application is greatly attractive but challenging. Herein, unsymmetrically coordinated Zn-N3O SAC with ultrahigh-loading of Zn up to 11.34 wt% is synthesized by means of a pre-adsorption-anchoring and pyrolysis approach. The strong adsorption of Zn ions by polypyrrole (PPy) and its inherent N/O source, coupled with the anchoring effect of ZIF-8 on Zn ions, is conducive to direct bonding between N/O atoms and Zn ions and the formation of high-loading atomic-scale Zn-N3O moieties, which are favorable for H2O2 production with a high selectivity up to nearly 100%. Density functional theory (DFT) computations further disclose that unsymmetrically coordinated Zn-N3O moieties tailor the ΔGOOH* near the peak of the volcano plot for 2e− ORR and therefore maximize the catalytic selectivity to form H2O2." @default.
- W4313201817 created "2023-01-06" @default.
- W4313201817 creator A5029524889 @default.
- W4313201817 creator A5037148185 @default.
- W4313201817 creator A5050873943 @default.
- W4313201817 creator A5053820816 @default.
- W4313201817 creator A5080995367 @default.
- W4313201817 creator A5091115474 @default.
- W4313201817 date "2023-01-01" @default.
- W4313201817 modified "2023-10-18" @default.
- W4313201817 title "Constructing ultrahigh-loading unsymmetrically coordinated Zn-N3O single-atom sites with efficient oxygen reduction for H2O2 production" @default.
- W4313201817 cites W2061367556 @default.
- W4313201817 cites W2070227796 @default.
- W4313201817 cites W2607231338 @default.
- W4313201817 cites W2765132906 @default.
- W4313201817 cites W2765774529 @default.
- W4313201817 cites W2782223820 @default.
- W4313201817 cites W2787972732 @default.
- W4313201817 cites W2795272585 @default.
- W4313201817 cites W2802378983 @default.
- W4313201817 cites W2810052757 @default.
- W4313201817 cites W2885206286 @default.
- W4313201817 cites W2886283368 @default.
- W4313201817 cites W2891982331 @default.
- W4313201817 cites W2903807505 @default.
- W4313201817 cites W2917431588 @default.
- W4313201817 cites W2924691801 @default.
- W4313201817 cites W2939405677 @default.
- W4313201817 cites W2966020790 @default.
- W4313201817 cites W2998215827 @default.
- W4313201817 cites W2999727704 @default.
- W4313201817 cites W3012441403 @default.
- W4313201817 cites W3025769129 @default.
- W4313201817 cites W3030808661 @default.
- W4313201817 cites W3034967233 @default.
- W4313201817 cites W3036377937 @default.
- W4313201817 cites W3080531864 @default.
- W4313201817 cites W3084502091 @default.
- W4313201817 cites W3106699956 @default.
- W4313201817 cites W3116329762 @default.
- W4313201817 cites W3157493048 @default.
- W4313201817 cites W3163242716 @default.
- W4313201817 cites W3163539100 @default.
- W4313201817 cites W3209928807 @default.
- W4313201817 cites W4225144483 @default.
- W4313201817 cites W4293379581 @default.
- W4313201817 doi "https://doi.org/10.1016/j.cej.2022.140721" @default.
- W4313201817 hasPublicationYear "2023" @default.
- W4313201817 type Work @default.
- W4313201817 citedByCount "10" @default.
- W4313201817 countsByYear W43132018172023 @default.
- W4313201817 crossrefType "journal-article" @default.
- W4313201817 hasAuthorship W4313201817A5029524889 @default.
- W4313201817 hasAuthorship W4313201817A5037148185 @default.
- W4313201817 hasAuthorship W4313201817A5050873943 @default.
- W4313201817 hasAuthorship W4313201817A5053820816 @default.
- W4313201817 hasAuthorship W4313201817A5080995367 @default.
- W4313201817 hasAuthorship W4313201817A5091115474 @default.
- W4313201817 hasConcept C104779481 @default.
- W4313201817 hasConcept C118792377 @default.
- W4313201817 hasConcept C140205800 @default.
- W4313201817 hasConcept C145148216 @default.
- W4313201817 hasConcept C147597530 @default.
- W4313201817 hasConcept C147789679 @default.
- W4313201817 hasConcept C149635348 @default.
- W4313201817 hasConcept C150394285 @default.
- W4313201817 hasConcept C152365726 @default.
- W4313201817 hasConcept C159985019 @default.
- W4313201817 hasConcept C161790260 @default.
- W4313201817 hasConcept C178790620 @default.
- W4313201817 hasConcept C179104552 @default.
- W4313201817 hasConcept C185592680 @default.
- W4313201817 hasConcept C192562407 @default.
- W4313201817 hasConcept C199164860 @default.
- W4313201817 hasConcept C41008148 @default.
- W4313201817 hasConcept C58312451 @default.
- W4313201817 hasConceptScore W4313201817C104779481 @default.
- W4313201817 hasConceptScore W4313201817C118792377 @default.
- W4313201817 hasConceptScore W4313201817C140205800 @default.
- W4313201817 hasConceptScore W4313201817C145148216 @default.
- W4313201817 hasConceptScore W4313201817C147597530 @default.
- W4313201817 hasConceptScore W4313201817C147789679 @default.
- W4313201817 hasConceptScore W4313201817C149635348 @default.
- W4313201817 hasConceptScore W4313201817C150394285 @default.
- W4313201817 hasConceptScore W4313201817C152365726 @default.
- W4313201817 hasConceptScore W4313201817C159985019 @default.
- W4313201817 hasConceptScore W4313201817C161790260 @default.
- W4313201817 hasConceptScore W4313201817C178790620 @default.
- W4313201817 hasConceptScore W4313201817C179104552 @default.
- W4313201817 hasConceptScore W4313201817C185592680 @default.
- W4313201817 hasConceptScore W4313201817C192562407 @default.
- W4313201817 hasConceptScore W4313201817C199164860 @default.
- W4313201817 hasConceptScore W4313201817C41008148 @default.
- W4313201817 hasConceptScore W4313201817C58312451 @default.
- W4313201817 hasFunder F4320321001 @default.
- W4313201817 hasLocation W43132018171 @default.
- W4313201817 hasOpenAccess W4313201817 @default.
- W4313201817 hasPrimaryLocation W43132018171 @default.