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- W4313201968 endingPage "122299" @default.
- W4313201968 startingPage "122299" @default.
- W4313201968 abstract "The chemical conversion of CO2 into hydrocarbon fuels and chemicals using green hydrogen not only utilizes abundant CO2 as a carbon feedstock but also enables the storage of hydrogen. Herein, we investigate the direct hydrogenation of CO2 to gasoline and olefins over a series of bifunctional iron-zeolite tandem catalysts operated at high temperatures (> 300 ℃). This process may efficiently utilize CO2 discharged from industrial combustion and green H2 produced by solid oxide electrolytic cells (SOEC). The optimized FeMnK+H-ZSM-5 catalyst offers a 70% selectivity of C5−C11 range hydrocarbons together with a 17% selectivity of C2−C4 lower olefins at 320 °C. The CO2 conversion levels and the aromatics contents could be greatly enhanced as the temperature increases from 320 ℃ to 400 ℃. The hydrocarbon distribution is mainly determined by the micropore size of the zeolites. The dynamic evolution of bifunctional catalysts and its impact on bifunctional catalysis was systematically investigated." @default.
- W4313201968 created "2023-01-06" @default.
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- W4313201968 date "2023-05-01" @default.
- W4313201968 modified "2023-10-18" @default.
- W4313201968 title "Direct conversion of carbon dioxide into liquid fuels and chemicals by coupling green hydrogen at high temperature" @default.
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- W4313201968 doi "https://doi.org/10.1016/j.apcatb.2022.122299" @default.
- W4313201968 hasPublicationYear "2023" @default.
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