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- W4313236978 endingPage "1209" @default.
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- W4313236978 abstract "Fast-charging lithium-ion batteries (LIBs) have been severely hampered by the slow development of their electrolytes. Herein, we demonstrate that the size effect of solvent sheath would pose a great effect on the fast-charging performance of LIBs. Three similar ethers, including diethyl ether (DEE), dipropyl ether (DPE), and dibutyl ether (DBE), were mixed with 1,1,2,2-tetrafluoroethyl-2,2,3,3-tetrafluoropropyl ether (TTE) and lithium bis(fluorosulfonyl)imide (1 M) to form an electrolyte for fast-charging LIBs, respectively. The results showed that it is more difficult to form ternary graphite intercalation compounds (GICs) in the electrolyte with a larger solvation sheath. The DEE electrolyte can form stable GICs and generate an inner LiF-rich solid electrolyte interphase (SEI), lowering the diffusion barrier of Li+. Therefore, the graphite anode powered by the DEE electrolyte can maintain a capacity of 190 mAh g-1 at 4 C after 500 cycles. This kind of size effect of solvation sheath is also applicable to lithium metal batteries." @default.
- W4313236978 created "2023-01-06" @default.
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- W4313236978 date "2022-12-28" @default.
- W4313236978 modified "2023-10-17" @default.
- W4313236978 title "Inner Lithium Fluoride (LiF)-Rich Solid Electrolyte Interphase Enabled by a Smaller Solvation Sheath for Fast-Charging Lithium Batteries" @default.
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- W4313236978 doi "https://doi.org/10.1021/acsami.2c17628" @default.
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